The density of helium bubbles in implanted materials

Results from VUV absorption and EEL spectroscopy.

S. E. Donnelly, A. A. Lucas, J. P. Vigneron, J. C. Rife

Research output: Contribution to journalConference article

21 Citations (Scopus)

Abstract

The novel application of vacuum ultra-violet absorption spectroscopy and electron energy loss spectroscopy to helium bubbles in metals is presented. These measurements, carried out on thin aluminum films containing different concentrations of helium and various bubble size distributions, were aimed at determining the density (and thus pressure) of helium in bubbles by observing the shift and broadening of the 1S-2P transition in the helium. The data coupled with a theoretical model developed by the authors indicate densities as high as 10**2**3 He cm** minus **3 for specimens containing small bubbles. Data are also presented on the effect that annealing and cooling have on these spectra. The annealing experiments give rise to fairly complex changes in absorption peak structure but with a general shift towards the unperturbed resonance line. The cooling experiment gives rise to a further shift and a narrowing of the absorption spectrum on cooling to 77 K which is tentatively identified as the liquid/solid transition in the helium. Finally, a fluorescence spectrum of an Al/He specimen excited with low energy electrons is presented.

Original languageEnglish
Pages (from-to)337-347
Number of pages11
JournalRadiation Effects
Volume78
Issue number1-4
DOIs
Publication statusPublished - 1 Jan 1983
Externally publishedYes
EventInternational Symposium on Fundamental Aspects of Helium in Materials - Julich, Germany
Duration: 21 Sep 198224 Sep 1982

Fingerprint

Helium
absorption spectroscopy
bubbles
helium
Spectroscopy
spectroscopy
Cooling
cooling
shift
Annealing
electron energy
annealing
ultraviolet absorption
Electron energy loss spectroscopy
Ultraviolet spectroscopy
Aluminum
Absorption spectroscopy
resonance lines
Absorption spectra
energy dissipation

Cite this

Donnelly, S. E. ; Lucas, A. A. ; Vigneron, J. P. ; Rife, J. C. / The density of helium bubbles in implanted materials : Results from VUV absorption and EEL spectroscopy. In: Radiation Effects. 1983 ; Vol. 78, No. 1-4. pp. 337-347.
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abstract = "The novel application of vacuum ultra-violet absorption spectroscopy and electron energy loss spectroscopy to helium bubbles in metals is presented. These measurements, carried out on thin aluminum films containing different concentrations of helium and various bubble size distributions, were aimed at determining the density (and thus pressure) of helium in bubbles by observing the shift and broadening of the 1S-2P transition in the helium. The data coupled with a theoretical model developed by the authors indicate densities as high as 10**2**3 He cm** minus **3 for specimens containing small bubbles. Data are also presented on the effect that annealing and cooling have on these spectra. The annealing experiments give rise to fairly complex changes in absorption peak structure but with a general shift towards the unperturbed resonance line. The cooling experiment gives rise to a further shift and a narrowing of the absorption spectrum on cooling to 77 K which is tentatively identified as the liquid/solid transition in the helium. Finally, a fluorescence spectrum of an Al/He specimen excited with low energy electrons is presented.",
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The density of helium bubbles in implanted materials : Results from VUV absorption and EEL spectroscopy. / Donnelly, S. E.; Lucas, A. A.; Vigneron, J. P.; Rife, J. C.

In: Radiation Effects, Vol. 78, No. 1-4, 01.01.1983, p. 337-347.

Research output: Contribution to journalConference article

TY - JOUR

T1 - The density of helium bubbles in implanted materials

T2 - Results from VUV absorption and EEL spectroscopy.

AU - Donnelly, S. E.

AU - Lucas, A. A.

AU - Vigneron, J. P.

AU - Rife, J. C.

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AB - The novel application of vacuum ultra-violet absorption spectroscopy and electron energy loss spectroscopy to helium bubbles in metals is presented. These measurements, carried out on thin aluminum films containing different concentrations of helium and various bubble size distributions, were aimed at determining the density (and thus pressure) of helium in bubbles by observing the shift and broadening of the 1S-2P transition in the helium. The data coupled with a theoretical model developed by the authors indicate densities as high as 10**2**3 He cm** minus **3 for specimens containing small bubbles. Data are also presented on the effect that annealing and cooling have on these spectra. The annealing experiments give rise to fairly complex changes in absorption peak structure but with a general shift towards the unperturbed resonance line. The cooling experiment gives rise to a further shift and a narrowing of the absorption spectrum on cooling to 77 K which is tentatively identified as the liquid/solid transition in the helium. Finally, a fluorescence spectrum of an Al/He specimen excited with low energy electrons is presented.

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